\u6709\u673a\u950c\u87af\u5408\u7269\uff0c\u65e0\u679d\u6676\u7684\u950c\u8d1f\u6781<\/strong><\/a><\/p>\n\u6c34\u7cfb\u950c\u91d1\u5c5e\u7535\u6c60\u7531\u4e8e\u4e25\u91cd\u7684\u6c34\u8150\u8680\u548c\u679d\u6676\u751f\u957f\uff0c\u5bfc\u81f4\u7535\u6c60\u5feb\u901f\u5faa\u73af\u964d\u89e3\u3002<\/p>\n
\u4e3a\u89e3\u51b3\u8fd9\u4e9b\u95ee\u9898\uff0c\u4e2d\u5357\u5927\u5b66Yuejiao Chen\uff0cLibao Chen\u5728\u950c\uff08Zn\uff09\u91d1\u5c5e\u8868\u9762\u8bbe\u8ba1\u4e86\u4e00\u79cd\u5177\u6709\u826f\u597d\u4eb2\u950c\u6027\u80fd\u548c\u7279\u6b8a\u7eb3\u7c73\u7ea7\u4e09\u7ef4\uff083D\uff09\u9897\u7c92\u7ed3\u6784\u7684\u9ad8\u6297\u6c34\u6027Znx-\u4e8c\u4e59\u70ef\u4e09\u80fa\u4e94(\u4e9a\u7532\u57fa\u81a6\u9178)\u754c\u9762\u5c42\u3002<\/p>\n
<\/p>\n
\u6587\u7ae0\u8981\u70b9<\/p>\n
1\uff09\u5b9e\u9a8c\u7ed3\u679c\u7ed3\u5408\u7406\u8bba\u5206\u6790\u548cCOMSOL\u6a21\u62df\u7ed3\u679c\u8868\u660e\uff0c\u8fd9\u79cd\u950c\u57fa\u6709\u673a\u914d\u5408\u7269\u4e2d\u7684\u758f\u6c34\u57fa\u56e2\u662f\u9632\u6b62H2O\u5bf9Zn\u8d1f\u6781\u8868\u9762\u8fdb\u884c\u7834\u574f\u7684\u51b3\u5b9a\u6027\u56e0\u7d20\u3002\u540c\u65f6\uff0c\u4e9a\u7532\u57fa\u81a6\u9178\u57fa\u4e0e\u950c\u7684\u76f8\u4e92\u4f5c\u7528\u5f62\u6210\u5927\u91cf\u7684\u950c\u79bb\u5b50\u5438\u5f15\u4f4d\uff0c\u4e3a\u950c\u79bb\u5b50\u7684\u5feb\u901f\u5438\u9644\u548c\u8fc1\u79fb\u63d0\u4f9b\u4e86\u79bb\u5b50\u901a\u9053\u3002\u800c\u8868\u9762\u53d1\u8fbe\u7684\u7eb3\u7c73\u9897\u7c92\u7ed3\u6784\u5bfc\u81f4\u950c\u79bb\u5b50\u901a\u91cf\u91cd\u65b0\u5206\u5e03\uff0c\u8868\u9762Zn\u6c89\u79ef\u5747\u5300\u81f4\u5bc6\u3002<\/p>\n
2\uff09\u5728\u534f\u540c\u4f5c\u7528\u4e0b\uff0c\u8fd9\u79cd\u4fee\u9970\u7684Zn\u8d1f\u6781\u5177\u6709\u957f\u8fbe1300 h\u7684\u5faa\u73af\u5bff\u547d\uff0c\u57285 mA cm\u22122\u5904\u6709\u8f83\u4f4e\u7684\u6781\u5316\u7535\u538b\u3002\u6b64\u5916\uff0c\u7814\u7a76\u4eba\u5458\u8fd8\u5c55\u793a\u4e86\u57fa\u4e8e\u8be5\u8d1f\u6781\u7ec4\u88c5\u7684\u5168\u7535\u6c60\u6c60\uff08\u5305\u62ecZn\/\/V2O5\u548cZn\/\/MnO2\u7535\u6c60\uff09\u3002<\/p>\n
\u8be5\u5de5\u4f5c\u901a\u8fc7\u7ed3\u6784\u8bbe\u8ba1\u548c\u5728\u8868\u9762\u6784\u5efa\u4fdd\u62a4\u5c42\u4e24\u4e2a\u6982\u5ff5\u7684\u7ed3\u5408\uff0c\u63d0\u4f9b\u4e86\u4e00\u6761\u7b80\u5355\u3001\u4f4e\u6210\u672c\u3001\u9ad8\u6548\u7684\u9014\u5f84\u6765\u5236\u5907\u9ad8\u6027\u80fd\u7684\u950c\u8d1f\u6781\uff0c\u4ece\u800c\u4e3a\u84ec\u52c3\u53d1\u5c55\u7684\u6c34\u7cfb\u950c\u91d1\u5c5e\u7535\u6c60\u63d0\u4f9b\u4e86\u4e00\u6761\u9014\u5f84\u3002<\/p>\n
<\/p>\n
2<\/p>\n
\u6709\u673a\u5fae\u91cf\u7684\u4f18\u52bf<\/p>\n
2.1 \u751f\u7269\u5229\u7528\u6548\u4ef7\u9ad8<\/p>\n
\u6709\u673a\u5fae\u91cf\u5143\u7d20\u4e0e\u65e0\u673a\u5fae\u91cf\u5143\u7d20\u76f8\u6bd4\uff0c\u6709\u673a\u5fae\u91cf\u5143\u7d20\u7684\u751f\u7269\u5229\u7528\u7387\u8f83\u9ad8\u3002\u4e3b\u8981\u662f\u56e0\u4e3a\u4e00\u822c\u7684\u5fae\u91cf\u5143\u7d20\u65e0\u673a\u76d0\u548c\u6709\u673a\u76d0\u88ab\u52a8\u7269\u4f53\u6444\u5165\u540e\uff0c\u5fc5\u987b\u5148\u8981\u501f\u52a9\u8f85\u9176\u7684\u4f5c\u7528\uff0c\u4e0e\u6c28\u57fa\u9178\u6216\u8005\u5176\u4ed6\u7269\u8d28\u5f62\u6210\u87af\u5408\u7269\u6216\u7edc\u5408\u7269\uff0c\u624d\u80fd\u591f\u88ab\u673a\u4f53\u5438\u6536\u3002\u5438\u6536\u540e\u7684\u91d1\u5c5e\u5143\u7d20\u4e0e\u86cb\u767d\u8d28\u7ed3\u5408\u88ab\u8fd0\u9001\u5230\u673a\u4f53\u6240\u9700\u8981\u7684\u90e8\u4f4d\u65f6\u624d\u80fd\u53d1\u6325\u529f\u6548\u3002\u86cb\u6c28\u9178\u950c\u3001\u86cb\u6c28\u9178\u94dc\u7b49\u6c28\u57fa\u9178\u87af\u5408\u7269\u6216\u7edc\u5408\u7269\u662f\u52a8\u7269\u4f53\u5438\u6536\u548c\u8f6c\u8fd0\u91d1\u5c5e\u79bb\u5b50\u7684\u4e3b\u8981\u5f62\u5f0f\uff0c\u4e5f\u662f\u52a8\u7269\u4f53\u5185\u5408\u6210\u86cb\u767d\u8fc7\u7a0b\u4e3b\u8981\u7684\u4e2d\u95f4\u4ea7\u7269\uff0c\u91c7\u7528\u8be5\u5f62\u5f0f\u4e0d\u4ec5\u5438\u6536\u5feb\uff0c\u800c\u4e14\u80fd\u591f\u51cf\u5c11\u8bb8\u591a\u751f\u5316\u8fc7\u7a0b\uff0c\u8282\u7ea6\u80fd\u91cf\u7684\u6d88\u8017\uff0c\u4ece\u800c\u4f7f\u5176\u5177\u6709\u8f83\u9ad8\u7684\u751f\u7269\u5b66\u6548\u4ef7\u3002\u53e6\u5916\uff0c\u52a8\u7269\u4f53\u5185\u5b58\u5728\u5fc5\u9700\u6c28\u57fa\u9178\u5e93\uff0c\u914d\u4f53\u4e3a\u5fc5\u9700\u6c28\u57fa\u9178\u7684\u6709\u673a\u5fae\u91cf\u5143\u7d20\u66f4\u5bb9\u6613\u4ee5\u6c28\u57fa\u9178\u6216\u5c0f\u80bd\u7684\u5f62\u5f0f\u50a8\u85cf\u5728\u4f53\u5185\uff0c\u9632\u6b62\u88ab\u5feb\u901f\u4ee3\u8c22\uff0c\u4ece\u800c\u589e\u52a0\u52a8\u7269\u5fae\u91cf\u5143\u7d20\u4f53\u8d2e\u5907\u3002\u56e0\u6b64\uff0c\u76f8\u8f83\u4e8e\u65e0\u6781\u5fae\u91cf\u5143\u7d20\uff0c\u6709\u673a\u5fae\u91cf\u5143\u7d20\u7528\u91cf\u66f4\u5c11\uff0c\u5b89\u5168\u6027\u548c\u6548\u76ca\u66f4\u9ad8\u3002<\/p>\n
2.2 \u51cf\u5c11\u77ff\u7269\u5143\u7d20\u76f8\u4e92\u62ee\u6297<\/p>\n
\u65e0\u673a\u5fae\u91cf\u5143\u7d20\u5177\u6709\u4e0d\u7a33\u5b9a\u548c\u6613\u7ed3\u5408\u7684\u7279\u70b9\uff0c\u53d1\u751f\u76f8\u4e92\u4f5c\u7528\u7684\u53ef\u80fd\u6027\u8981\u6bd4\u5176\u4ed6\u7269\u8d28\u5bb9\u6613\u3002\u8fd9\u4e9b\u4f5c\u7528\u53d1\u751f\u5728\u9972\u6599\u4e4b\u95f4\uff0c\u5728\u6d88\u5316\u9053\u7ec4\u7ec7\u548c\u7ec6\u80de\u4ee3\u8c22\u8fc7\u7a0b\u4e2d\u5fae\u91cf\u5143\u7d20\u4e4b\u95f4\u4ee5\u53ca\u4e0e\u5e38\u91cf\u5143\u7d20\u4e4b\u95f4\u5728\u5438\u6536\u6392\u6cc4\u3001\u8f6c\u8fd0\u4ee3\u8c22\u3001\u529f\u80fd\u53d1\u6325\u7b49\u8fc7\u7a0b\u4e2d\u5b58\u5728\u8bb8\u591a\u62ee\u6297\u3002\u8fd9\u62ee\u6297\u4f5c\u7528\u53d1\u751f\u5728\u6d88\u5316\u9053\u4e2d\u7684\u4e3b\u8981\u5f62\u5f0f\u662f\uff1a\u2460\u5143\u7d20\u95f4\u53d1\u751f\u7b80\u5355\u7684\u5316\u5b66\u53cd\u5e94\u3002\u5982\u65e5\u7cae\u5185\u9541\u8fc7\u591a\uff0c\u5728\u6d88\u5316\u9053\u5185\u53ef\u5f62\u6210\u78f7\u9178\u9541\uff0c\u4ece\u800c\u963b\u788d\u78f7\u7684\u5438\u6536\u3002\u2461\u88ab\u80f6\u4f53\u9897\u7c92\u5438\u9644\u3002\u5982\u94c1\u4e0e\u9530\u6709\u76f8\u540c\u7684\u7535\u5b50\u8f68\u9053 \u3001\u6784\u578b\u548c\u914d\u4f4d\u6570\uff0c\u53ef\u56fa\u5b9a\u4e8e\u975e\u6eb6\u6027\u7684\u9541\u76d0\u6216\u94dd\u76d0\u8868\u9762\uff0c\u4ece\u800c\u4f7f\u94c1\u4e0e\u9530\u5728\u6d88\u5316\u9053\u7684\u5438\u6536\u51cf\u5c11\u3002\u2462\u79bb\u5b50\u5728\u80a0\u58c1\u4e0a\u7ade\u4e89\u8f7d\u4f53\u3002\u94dc\u4e0e\u950c\u90fd\u662f\u5728\u5c0f\u80a0\u5438\u6536\uff0c\u5b83\u4eec\u5728\u91d1\u5c5e\u786b\u86cb\u767d\u6216\u80a0\u7c98\u819c\u4e2d\u53ef\u4e92\u76f8\u7ade\u4e89\u7ed3\u5408\u90e8\u4f4d\uff0c\u4ece\u800c\u5bfc\u81f4\u4e92\u76f8\u5438\u6536\u6291\u5236\u3002\u6709\u673a\u5fae\u91cf\u5143\u7d20\u5728\u52a8\u7269\u673a\u4f53\u5185\u7684\u5438\u6536\u4e0e\u65e0\u673a\u76d0\u4e0d\u540c\uff0c\u6c28\u57fa\u9178\u53ca\u86cb\u767d\u87af\u5408\u7269\u5229\u7528\u80bd\u548c\u6c28\u57fa\u9178\u7684\u5438\u6536\u673a\u5236\uff0c\u4ee5\u6c28\u57fa\u9178\u6216\u80bd\u7684\u5f62\u5f0f\u88ab\u5438\u6536\u3002\u56e0\u6b64\u4e0d\u5b58\u5728\u76f8\u4e92\u62ee\u6297\u7684\u4f5c\u7528\uff0c\u4ece\u800c\u7528\u91cf\u66f4\u53ef\u63a7\uff0c\u66f4\u5408\u7406\u3002<\/p>\n
<\/p>\n
2.3 \u907f\u514d\u4e0e\u9972\u6599\u4e2d\u7684\u6297\u8425\u517b\u56e0\u5b50\u62ee\u6297<\/p>\n
\u65e0\u673a\u5fae\u91cf\u5143\u7d20\u5728\u52a8\u7269\u80a0\u9053\u5185\u80fd\u4e0e\u7ea4\u7ef4\u3001\u690d\u9178\u7b49\u7ed3\u5408\u5728\u4e00\u8d77\u5f62\u6210\u7a33\u5b9a\u7684\u7ed3\u6784\uff0c\u5982\u4e2d\u6027\u6d17\u6da4\u7ea4\u7ef4\uff08NDF\uff09\u80fd\u4e0e\u4e8c\u4ef7\u94c1\u7ed3\u5408\u5f71\u54cd\u5438\u6536\uff1b\u690d\u9178\u80fd\u4e0e\u4e8c\u4ef7\u7684\u94dc\u3001\u94c1\u3001\u950c\u7ed3\u5408\u751f\u6210\u6c89\u6dc0\uff0c\u4ece\u800c\u964d\u4f4e\u5438\u6536\uff1b\u800c\u6709\u673a\u5fae\u91cf\u5143\u7d20\u4e2d\u7684\u91d1\u5c5e\u79bb\u5b50\u4f4d\u4e8e\u87af\u5408\u7269\u4e2d\u5fc3\uff0c\u4e0e\u914d\u4f53\u901a\u8fc7\u914d\u4f4d\u548c\u5171\u4ef7\u952e\u7ed3\u5408\u540e\uff0c\u5176\u5206\u5b50\u5185\u7535\u8377\u8d8b\u4e8e\u4e2d\u6027\uff0c\u5f62\u6210\u7a33\u5b9a\u7ed3\u6784\uff0c\u4e0d\u4f1a\u88ab\u65e5\u7cae\u4e2d\u7684\u6297\u8425\u517b\u56e0\u5b50\u7ed3\u5408\u800c\u5f71\u54cd\u5438\u6536\u3002<\/p>\n
2.4 \u6297\u6c27\u5316\u548c\u63d0\u9ad8\u514d\u75ab\u7684\u80fd\u529b\u66f4\u5f3a<\/p>\n
\u8fd1\u5e74\u6765\u5927\u91cf\u7684\u7814\u7a76\u8868\u660e\uff0c\u6709\u673a\u5fae\u91cf\u5143\u7d20\u5728\u63d0\u9ad8\u514d\u75ab\u529f\u80fd\uff0c\u6539\u5584\u80a0\u9053\u5065\u5eb7\u548c\u51cf\u5c11\u5e94\u6fc0\u65b9\u9762\u4f18\u4e8e\u65e0\u673a\u76d0\u5fae\u91cf\u5143\u7d20\u3002\u80fd\u591f\u589e\u5f3a\u673a\u4f53\u7684\u6297\u75bc\u75db\u80fd\u529b\uff0c\u5927\u9650\u5ea6\u7684\u63d0\u9ad8\u673a\u4f53\u7684\u514d\u75ab\u5e94\u7b54\u53cd\u5e94\uff0c\u4fc3\u8fdb\u7ec6\u80de\u514d\u75ab\u548c\u4f53\u6db2\u514d\u75ab\uff0c\u53d1\u6325\u6297\u5e94\u6fc0\u548c\u6297\u75c5\u7684\u4f5c\u7528\u3002<\/p>\n
2.5 \u5316\u5b66\u6027\u8d28\u7a33\u5b9a<\/p>\n
\u65e0\u673a\u76d0\u5206\u5b50\u4e2d\uff0c\u9634\u3001\u9633\u79bb\u5b50\u901a\u8fc7\u9759\u7535\u5f62\u6210\u4e0d\u591f\u7a33\u5b9a\u7684\u79bb\u5b50\u952e\uff0c\u6240\u4ee5\u6781\u6613\u4e0e\u5176\u4ed6\u7269\u8d28\u53d1\u751f\u5316\u5b66\u53cd\u5e94\uff0c\u5316\u5b66\u7ed3\u6784\u6781\u4e0d\u7a33\u5b9a\uff1b\u800c\u6709\u673a\u5fae\u91cf\u4ee5\u5fae\u91cf\u5143\u7d20\u79bb\u5b50\u4e3a\u4e2d\u5fc3\uff0c\u5c06\u6c28\u57fa\u9178\u4e2d\u7684\u6c27\u548c\u6c2e\u539f\u5b50\u5305\u88f9\u5728\u5fae\u91cf\u5143\u7d20\u7684\u5916\u9762\uff0c\u5c06\u5fae\u91cf\u5143\u7d20\u5c01\u95ed\u8d77\u6765\uff0c\u8fd9\u4f7f\u5f97\u5b83\u5177\u6709\u6bd4\u8f83\u7a33\u5b9a\u7684\u5316\u5b66\u6027\u8d28\uff0c\u4e5f\u4f7f\u5f97\u5206\u5b50\u5185\u7535\u8377\u8d8b\u4e8e\u4e2d\u6027\uff0c\u5728\u4f53\u5185\u53ef\u4ee5\u6709\u6548\u4fdd\u62a4\u91d1\u5c5e\u79bb\u5b50\uff0c\u4ece\u800c\u4f7f\u91d1\u5c5e\u79bb\u5b50\u907f\u514d\u4e0e\u80c3\u80a0\u9053\u4e2d\u7684\u80c3\u9178\u548c\u65e5\u7cae\u4e2d\u7684\u5176\u4ed6\u6210\u5206\u7b49\u7269\u8d28\u53d1\u751f\u4e0d\u826f\u53cd\u5e94\u3002\u5c24\u5176\u6c28\u57fa\u9178\u87af\u5408\u7269\u662f\u901a\u8fc7\u914d\u4f4d\u5171\u4ef7\u952e\u7ed3\u5408\uff0c\u5176\u7a33\u5b9a\u6027\u6bd4\u901a\u8fc7\u79bb\u5b50\u952e\u7ed3\u5408\u7684\u7edc\u5408\u7269\u66f4\u9ad8\u3002<\/p>\n
3<\/p>\n
\u7ed3\u675f\u8bed<\/p>\n
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